论文标题

晶体的极端紫外线高谐波的Attosond同步

Attosecond synchronization of extreme ultraviolet high harmonics from crystals

论文作者

Vampa, Giulio, Lu, Jian, You, Yong Sing, Baykusheva, Denitsa R., Wu, Mengxi, Liu, Hanzhe, Schafer, Kenneth J., Gaarde, Mette B., Reis, David A., Ghimire, Shambhu

论文摘要

强近红外(NIR)激光脉冲与宽带gap介电的相互作用在极端紫外线(XUV)波长范围内产生高谐波。这些观察结果开辟了固体中attsecond计量学的可能性,这将受益于对NIR激光场的单个谐波的发射时间的精确测量。在这里,我们表明,当从氧化镁晶体的输入表面检测到高野马,对XUV发射的双重探测表明,明确的同步在很大程度上与散装固体中电子孔回旋的半经典模型一致。另一方面,源自200 $ $ $ m厚的晶体的谐波的谐波谱图得到了强烈修饰,表明在传播过程中激光场畸变的影响。我们在XUV Energies上对亚周期电子和孔重新收集的跟踪与Attosecond脉冲的固态来源的发展有关。

The interaction of strong near-infrared (NIR) laser pulses with wide-bandgap dielectrics produces high harmonics in the extreme ultraviolet (XUV) wavelength range. These observations have opened up the possibility of attosecond metrology in solids, which would benefit from a precise measurement of the emission times of individual harmonics with respect to the NIR laser field. Here we show that, when high-harmonics are detected from the input surface of a magnesium oxide crystal, a bichromatic probing of the XUV emission shows a clear synchronization largely consistent with a semiclassical model of electron-hole recollisions in bulk solids. On the other hand, the bichromatic spectrogram of harmonics originating from the exit surface of the 200 $μ$m-thick crystal is strongly modified, indicating the influence of laser field distortions during propagation. Our tracking of sub-cycle electron and hole re-collisions at XUV energies is relevant to the development of solid-state sources of attosecond pulses.

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