论文标题
当地力量偶极子响应计算机眼镜中的统计力学
Statistical mechanics of local force dipole responses in computer glasses
论文作者
论文摘要
柔软的准化模式(QLM)普遍列出了从熔体中淬火的结构玻璃,据说涉及许多玻璃状异常,例如其导热性和特定热量的低温尺度,并在中等频率下进行声音衰减。在计算机眼镜中,QLM可以假设在狭窄的情况下谐波振动模式的形式,但是,QLM与其他低频模式(例如〜Phonons)的杂种会阻碍其在频率上的完整分布。以前克服该问题的研究表明,玻璃对局部力量偶极子的反应是其QLM的良好代理。因此,我们在这里研究了计算机玻璃中对局部力量偶极子的响应的统计机械特性,在大量的玻璃稳定性和各个空间维度上,目的是揭示QLMS频率尚无法完全分布的特性。我们发现,与QLMS频率$ω$的空间差异无关的通用分布(因此,它们的刚度$κ\!= \!ω^2 $),与对局部力偶极子偶极子偶极子偶极性偶极性的抗刚度的分布A(弱)依赖于空间压力。我们通过引入一个晶格模型来合理化这种依赖性,该晶格模型既包含QLM的真实空间曲线---与依赖性依赖性的长距离弹性字段相关联 - 及其频率的通用统计属性。最后,我们讨论了我们的发现与玻璃过渡问题的基本方面之间的可能联系,以及在超高玻璃的塑性活动中的有限尺寸效果。
Soft quasilocalized modes (QLMs) are universally featured by structural glasses quenched from a melt, and are supposedly involved in a number of glassy anomalies such as the low temperature scaling of their thermal conductivity and specific heat, and sound attenuation at intermediate frequencies. In computer glasses, QLMs may assume the form of harmonic vibrational modes under a narrow set of circumstances, however direct access to their full distribution over frequency is hindered by hybridizations of QLMs with other low-frequency modes (e.g.~phonons). Previous studies to overcome this issue have demonstrated that the response of a glass to local force dipoles serves as a good proxy for its QLMs; we therefore study here the statistical-mechanical properties of the responses to local force dipoles in computer glasses, over a large range of glass stabilities and in various spatial dimensions, with the goal of revealing properties of the yet-inaccessible full distribution of QLMs' frequencies. We find that, as opposed to the spatial-dimension-independent universal distribution of QLMs' frequencies $ω$ (and, consequently, also of their stiffness $κ\!=\!ω^2$), the distribution of stiffnesses associated with responses to local force dipoles features a (weak) dependence on spatial dimension. We rationalize this dependence by introducing a lattice model that incorporates both the real-space profiles of QLMs --- associated with dimension-dependent long-range elastic fields --- and the universal statistical properties of their frequencies. Finally, we discuss possible connections between our findings and basic aspects of the glass transition problem, and to finite-size effects in plastic activity of ultrastable glasses.