论文标题
稀量热气中多量子相干信号的理论
Theory of multiple quantum coherence signals in dilute thermal gases
论文作者
论文摘要
由于强烈的不均匀扩张,很难感知稀释热气中偶极 - 偶极相互作用的表现。最近的实验报告了这种相互作用在基于荧光检测的多量子相干性(MQC)信号中的签名,迄今无法解释的许多特征特征。我们在稀的热气体中开发了MQC的原始开放量子系统理论,这使我们能够解决此难题。我们的理论说明了原子偶极子的矢量特征以及驱动任意强度的激光脉冲,包括偶极子之间的远场耦合,偶极子在稀释的集合中占上风,并通过疾病平均值有效地融合了原子运动。我们表明,集体衰减过程 - 在使用偶极相互作用的静电形式的先前治疗中被忽略 - 在MQC信号的出现中起着关键作用。
Manifestations of dipole-dipole interactions in dilute thermal gases are difficult to sense because of strong inhomogeneous broadening. Recent experiments reported signatures of such interactions in fluorescence detection-based measurements of multiple quantum coherence (MQC) signals, with many characteristic features hitherto unexplained. We develop an original open quantum systems theory of MQC in dilute thermal gases, which allows us to resolve this conundrum. Our theory accounts for the vector character of the atomic dipoles as well as for driving laser pulses of arbitrary strength, includes the far-field coupling between the dipoles, which prevails in dilute ensembles, and effectively incorporates atomic motion via a disorder average. We show that collective decay processes -- which were ignored in previous treatments employing the electrostatic form of dipolar interactions -- play a key role in the emergence of MQC signals.