论文标题
用于电子泵的紫外线源的Algan/Aln量子点超级晶格的内部量子效率
Internal quantum efficiency of AlGaN/AlN quantum dot superlattices for electron-pumped ultraviolet sources
论文作者
论文摘要
在本文中,我们描述了Alxga1-Xn/Aln(X = 0,0.1)的530 nm厚度超晶格(100个周期)的生长和表征,用于应用电子束式紫外紫外线灯的活性区域。高密度(> 10E11 cm-2)量子点层通过分子束外延沉积,我们探索了生长过程中III/V比的影响对其光学性能的影响。该研究认为在室温下排放的结构在244-335 nm范围内发射,相对线宽在6-11%的范围内,这主要是由于QD直径分散体固有的自组装生长。在电子泵送下,对于低于9 kV的加速度电压,发射效率保持恒定。该阈值与超晶格的总厚度和电子束的穿透深度的相关性证实了沿生长轴的纳米结构的均匀性。在阈值以下,发射强度与注射电流线性缩放。内部量子效率在低注入时的特征是在非辐射过程中揭示了材料的特性,并在高注射过程中揭示了在操作条件下模拟载体注入的高注射。在与III/V比<0.75合成的量子点中,内部量子效率从低注射量到泵浦功率密度高达200 kW/cm2的50%约为50%,是第一种呈现这种稳定行为的纳米结构。
In this paper, we describe the growth and characterization of 530-nm-thick superlattices (100 periods) of AlxGa1-xN/AlN (x = 0, 0.1) Stranski-Krastanov quantum dots for application as the active region of electron-beam pumped ultraviolet lamps. Highly dense (>10e11 cm-2) quantum dot layers are deposited by molecular beam epitaxy, and we explore the effect of the III/V ratio during the growth process on their optical performance. The study considers structures emitting in the 244-335 nm range at room temperature, with a relative linewidth in the 6-11% range, mainly due to the QD diameter dispersion inherent in self-assembled growth. Under electron pumping, the emission efficiency remains constant for acceleration voltages below 9 kV. The correlation of this threshold with the total thickness of the superlattice and the penetration depth of the electron beam confirms the homogeneity of the nanostructures along the growth axis. Below the threshold, the emission intensity scales linearly with the injected current. The internal quantum efficiency is characterized at low injection, which reveals the material properties in terms of non-radiative processes, and high injection, which emulates carrier injection in operation conditions. In quantum dots synthesized with III/V ratio < 0.75, the internal quantum efficiency remains around 50% from low injection to pumping power densities as high as 200 kW/cm2, being the first kind of nanostructures that present such stable behaviour.