论文标题
通过电荷转移到铁电绝缘子的电荷转移,人工二维极性金属
Artificial two-dimensional polar metal by charge transfer to a ferroelectric insulator
论文作者
论文摘要
在单个系统中集成多个特性对于电子设备的连续开发至关重要。但是,某些物理特性本质上是相互排斥的。在这里,我们报告了两个看似相互排斥的属性极性和二维电导率的共存,以ba $ _ {0.2} $ sr $ _ {0.8} $ _3} $ _3 $ _3 $ thin fimss在laalo $ _3 $ _3 $ _2 $ _2 $ _ {0.2 $ _ {0.2} $ _ $ _ $ sr $ sr $ sr $ sr $ _ {0.8 〜3.2 nm ba $ _ {0.2} $ sr $ _ {0.8} $ tio $ _3 $薄膜的极性保留,二维移动载流子密度为每个单位电池〜0.05个电子。我们表明,由Laalo $ _3 $的内置电场与BA $ _ {0.2} $ SR $ _ {0.8} $ TIO $ _3 $之间的竞争产生的电子重建是负责此不寻常的二维导电阶段。通过电子重建在氧化物界面上利用互斥性质的一般概念可能适用于其他强相关的氧化物界面,从而为新型的纳米级材料打开了用于新型纳米电子学应用的新功能性纳米级材料。
Integrating multiple properties in a single system is crucial for the continuous developments in electronic devices. However, some physical properties are mutually exclusive in nature. Here, we report the coexistence of two seemingly mutually exclusive properties-polarity and two-dimensional conductivity-in ferroelectric Ba$_{0.2}$Sr$_{0.8}$TiO$_3$ thin films at the LaAlO$_3$/Ba$_{0.2}$Sr$_{0.8}$TiO$_3$ interface at room temperature. The polarity of a ~3.2 nm Ba$_{0.2}$Sr$_{0.8}$TiO$_3$ thin film is preserved with a two-dimensional mobile carrier density of ~0.05 electron per unit cell. We show that the electronic reconstruction resulting from the competition between the built-in electric field of LaAlO$_3$ and the polarization of Ba$_{0.2}$Sr$_{0.8}$TiO$_3$ is responsible for this unusual two-dimensional conducting polar phase. The general concept of exploiting mutually exclusive properties at oxide interfaces via electronic reconstruction may be applicable to other strongly-correlated oxide interfaces, thus opening windows to new functional nanoscale materials for applications in novel nanoelectronics.