论文标题
近晶相和不同密度的各向同性相之间接口的动力学模型
Model of the dynamics of an interface between a smectic phase and an isotropic phase of different density
论文作者
论文摘要
软调制相已显示出具有复杂的形态跃迁,其中均值和高斯曲率诱导的层重塑起主要作用。在热处理下的近晶膜中,这种情况就是这种情况,可以将焦点锥体重塑为锥形金字塔和同心环结构。我们基于对近视时期的早期研究,这是两相配置,其中界面的扩散演化是由曲率驱动的,而大规模运输则被忽略。在这里,我们明确考虑通过共存的各向同性流体相的质量转移,以及界面和界面和结果流的流体动力应力。通过采用Coleman-Noll程序,我们得出了一个相位模型,该模型是耦合到订单参数的近晶层的不同密度场。所得方程决定了具有不同密度的调制相和各向同性流体相之间界面的演变,并且它们在界面区域和拓扑转变中捕获可压缩性效应。我们首先通过检查界面横向模式的分散关系来验证管理方程的数值实现。由于流体动力效应,反向衰减速率显示为缩放为$ q^{2} $($ q $是扰动的波数),而不是预期的扩散衰减的$ q^{4} $。然后,通过将方程式在时间前进,我们研究了扭曲的层和焦点锥体上的流体流,并显示界面应力和密度对比度如何显着确定流动的结构以及构型的演变。
Soft modulated phases have been shown to undergo complex morphological transitions, in which layer remodeling induced by mean and Gaussian curvatures plays a major role. This is the case in smectic films under thermal treatment, where focal conics can be reshaped into conical pyramids and concentric ring structures. We build on earlier research on a smectic-isotropic, two phase configuration in which diffusive evolution of the interface was driven by curvature, while mass transport was neglected. Here, we explicitly consider evaporation-condensation processes in a smectic phase with mass transport through a coexisting isotropic fluid phase, as well as the hydrodynamic stresses at the interface and the resulting flows. By employing the Coleman-Noll procedure, we derive a phase-field model that accounts for a varying density field coupled to smectic layering of the order parameter. The resulting equations govern the evolution of an interface between a modulated phase and an isotropic fluid phase with distinct densities, and they capture compressibility effects in the interfacial region and topological transitions. We first verify a numerical implementation of the governing equations by examining the dispersion relation for interfacial transverse modes. The inverse decay rate is shown to scale as $Q^{2}$ ($Q$ is the wavenumber of the perturbation) due to hydrodynamic effects, instead of the $Q^{4}$ expected for diffusive decay. Then, by integrating the equations forward in time, we investigate fluid flow on distorted layers and focal conics, and show how interfacial stresses and density contrast significantly determine the structure of the flow and the evolution of the configuration.