论文标题

时间分辨一致镜检查的高重复速率attosent Light源

A high-repetition rate attosecond light source for time-resolved coincidencespectroscopy

论文作者

Mikaelsson, Sara, Vogelsang, Jan, Guo, Chen, Sytcevich, Ivan, Viotti, Anne-Lise, Langer, Fabian, Cheng, Yu-Chen, Nandi, Saikat, Jin, Wenjie, Olofsson, Anna, Weissenbilder, Robin, Mauritsson, Johan, L'Huillier, Anne, Gisselbrecht, Mathieu, Arnold, Cord L.

论文摘要

通过气体中的高阶谐波产生产生的Attsond脉冲已成功地用于观察原子,分子和固态系统中的超快,次秒电子动力学。然而,当今典型的ATTSENT来源通常会因其低重复率和由此产生的统计数据不足而受到损害,尤其是当每次射击的可检测事件数量受到限制时。对于必须在巧合中检测到几种反应产物的实验,以及空间充电效应损害光谱和空间分辨率的表面科学应用。 在这项工作中,我们提出了一个在200 kHz下运行的Attsond Light源,该光源开辟了对以前无法访问的现象,无法访问Attsosend Interfermetric和Spectroscopic技术。我们方法的关键是高重复速率的组合,几乎没有周期的激光源,一个专门设计的气体目标,可用于高效高谐波生成,一种被动稳定的泵探针干涉仪和高级的3D光电/离子动量探测器。到目前为止,迄今为止,在迄今为止的大多数实验中都使用了单一的脉冲或长杆脉冲进行,但我们探索了迄今为止主要被忽略的中间状态,短列车仅通过少量attsosecond脉冲组成。这为未来对强相关电子的动态演变的研究开放。

Attosecond pulses, produced through high-order harmonic generation in gases, have been successfully used for observing ultrafast, sub-femtosecond electron dynamics in atoms, molecules and solid state systems. Today's typical attosecond sources, however, are often impaired by their low repetition rate and the resulting insufficient statistics, especially when the number of detectable events per shot is limited. This is the case for experiments where several reaction products must be detected in coincidence, and for surface science applications where space-charge effects compromise spectral and spatial resolution. In this work, we present an attosecond light source operating at 200 kHz, which opens up the exploration of phenomena previously inaccessible to attosecond interferometric and spectroscopic techniques. Key to our approach is the combination of a high repetition rate, few-cycle laser source, a specially designed gas target for efficient high harmonic generation, a passively and actively stabilized pump-probe interferometer and an advanced 3D photoelectron/ion momentum detector. While most experiments in the field of attosecond science so far have been performed with either single attosecond pulses or long trains of pulses, we explore the hitherto mostly overlooked intermediate regime with short trains consisting of only a few attosecond pulses.e also present the first coincidence measurement of single-photon double ionization of helium with full angular resolution, using an attosecond source. This opens up for future studies of the dynamic evolution of strongly correlated electrons.

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