论文标题

在室温下单层半导体微腔中的超阈值极化偏心凝结物

Ultralow Threshold Polariton Condensate in a Monolayer Semiconductor Microcavity at Room Temperature

论文作者

Zhao, Jiaxin, Su, Rui, Fieramosca, Antonio, Zhao, Weijie, Du, Wei, Liu, Xue, Diederichs, Carole, Sanvitto, Daniele, Liew, Timothy C. H., Xiong, Qihua

论文摘要

原子上薄的过渡金属二分法具有依赖山谷的功能,通常仅在Crogenic温度下可用,受到各种山谷去极化散射的约束。通过相干叠加的激子和微腔光子形成激子极化子的形成潜在地利用了新型ValleyTronics设备的山谷极化偏振子相互作用。在室温下,TMDS微腔内已经证明了强大的EPS,但是,连贯的极性激光和冷凝水仍然难以捉摸。本文中,我们首次证明了在室温下TMD微腔中EP冷凝的实现。连续波泵送EP的凝结和激光,并通过对基态的宏观占用所证明的超级阈值激光,从而经历了发射的非线性增加和连续的Blueshift,空间相干性的堆积,以及一个失调的控制阈值。我们的工作迈出了至关重要的一步,朝着利用在室温下具有山谷功能的非线性极化层相互作用和极化设备。

Atomically thin transition metal dichalcogenides possess valley dependent functionalities that are usually available only at crogenic temperatures, constrained by various valley depolarization scatterings. The formation of exciton polaritons by coherently superimposing excitons and microcavity photons potentially harnesses the valley polarized polariton polariton interactions for novel valleytronics devices. Robust EPs have been demonstrated at room temperature in TMDs microcavity, however, the coherent polariton lasing and condensation remain elusive. Herein, we demonstrate for the first time the realization of EP condensation in a TMD microcavity at room temperature. The continuous wave pumped EP condensation and lasing with ultralow thresholdsis evidenced by the macroscopic occupation of the ground state, that undergoes a nonlinear increase of the emission and a continuous blueshift, a build up of spatial coherence, and a detuning-controlled threshold. Our work presents a critically important step towards exploiting nonlinear polariton polariton interactions and polaritonic devices with valley functionality at room temperature.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源