论文标题

扭曲双层石墨烯中的巨型二阶非线性

Giant second-order nonlinearity in twisted bilayer graphene

论文作者

Duan, Junxi, Jian, Yu, Gao, Yang, Peng, Huimin, Zhong, Jinrui, Feng, Qi, Yao, Yugui

论文摘要

在二阶响应方案中,只要系统是非中心对称的,霍尔电压就可以非零地不为零。有多种具有不同缩放规则的机制,这些机制有助于非线性霍尔效应(NLHE)。固有贡献与浆果曲率偶极子密切相关,并且最近已广泛研究。但是,对外部贡献的研究很少,尽管它可以以领先的顺序进入NLHE。在这里,我们报告了TBG中的巨型非线性转运响应,其中禁止内在机制。二阶非线性的大小和方向可以通过门电压有效调节。接近Moiré乐队的完整填充的二阶电导率的峰值达到8.76 $μmsv^{ - 1} $,四阶大于$ WTE_2 $中检测到的峰值。可以从非中心对称晶体中静态(库仑杂质)和动态障碍(colomb杂质)和动态障碍(Phonon)的不对称散射的协作来理解观察到的巨型二阶非线性。它主要取决于1.7 k的杂质的偏斜碎片贡献。从缩放结果所建议的,来自声子的偏斜散射的耦合系数要大得多,并且与温度上升的杂质贡献一样重要。我们的观察结果表明,TBG在研究非线性反应和可能的整流应用中的潜力。

In the second-order response regime, the Hall voltage can be nonzero without breaking the time-reversal symmetry, as long as the system is noncentrosymmetric. There are multiple mechanisms with different scaling rules that contribute to the nonlinear Hall effect (NLHE). The intrinsic contribution is closely related to the Berry curvature dipole and has been extensively investigated recently. The study of the extrinsic contribution, however, is scarce, although it can enter the NLHE even in the leading order. Here, we report a giant nonlinear transport response in TBG, in which the intrinsic mechanism is forbidden. The magnitude and direction of the second-order nonlinearity can be effectively tuned by the gate voltage. The peak value of the second-order Hall conductivity close to the full filling of the moiré band reaches 8.76 $μmSV^{-1}$, four-order larger than those detected in $WTe_2$. The observed giant second-order nonlinearity can be understood from the collaboration of the asymmetric scattering of electrons off the static (Coulomb impurities) and dynamic disorders (phonons) in noncentrosymmetric crystals. It is mainly determined by the skew-scattering contribution from impurities at 1.7 K. The skew-scattering from phonons has a much larger coupling coefficient as suggested by the scaling results, and becomes as important as the impurity contribution as the temperature rises. Our observations demonstrate the potential of TBG in studying nonlinear response and possible rectification applications.

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