论文标题

二维半导体的光子发射工程的低成本等离子体平台

A low cost plasmonic platform for photon emission engineering of two dimensional semiconductors

论文作者

Singh, Anuj Kumar, Mandal, Kishor K, Gupta, Yashika, VS, Abhay Anand, Eswaramoorthy, Lekshmi, Kumar, Brijesh, Kala, Abhinav, Dixit, Saurabh, Achanta, Venu Gopal, Kumar, Anshuman

论文摘要

尽管2D材料的领域通过使高质量的样品便宜地访问,因此由于这些系统的原子性质较薄而使材料科学民主化,但几乎总是需要与纳米结构进行集成以获得大量的光学响应。传统上,这些纳米结构是通过电子束光刻或聚焦离子束铣削制造的,这些纳米片台化昂贵,大面积制造可能会进一步耗时。为了克服这个问题,我们报告了2D半导体在成本效益且大面积的纳米酮平台上的集成。我们表明,与非差异情况相比,我们的纳米酮结构的等离子模式导致单层WSE $ _2 $的光致发光(PL)增强大约八到十倍,与有限差分时间域模拟一致。激发功率依赖性测量结果表明,我们的纳米酮平台为工程提供了对发射的相对激子贡献的多功能途径。

Although the field of 2D materials has democratized materials science by making high quality samples accessible cheaply, due to the atomically thin nature of these systems, an integration with nanostructures is almost always required to obtain a significant optical response. Traditionally, these nanostructures are fabricated via electron beam lithography or focused ion beam milling, which are expensive and large area fabrication can be further time consuming. In order to overcome this problem, we report the integration of 2D semiconductors on a cost-effective and large area fabricated nanocone platform. We show that the plasmon modes of our nanocone structures lead to photoluminescence (PL) enhancement of monolayer WSe$_2$ by about eight to ten times compared to the non-plasmonic case, consistent with finite-difference time-domain simulations. Excitation power-dependent measurements reveal that our nanocone platform enables a versatile route to engineering the relative exciton trion contributions to the emission.

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