论文标题

非线性光学响应理论

Theory of nonlinear optical response

论文作者

Sheikhabadi, Amin Maleki, Bagheri, Zahra, Sadeghi, Ali

论文摘要

我们提出了一种一般形式主义,用于研究固体对弱无序晶体中电场的二阶光学响应,该晶体具有基于密度 - 矩阵运动方程,天生对疾病的近似处理以及散射速率的扩大到领先的非宽度顺序的散射速率,具有任意复杂的带状结构。我们工作的主要目的之一是实现广泛的运输理论应用,该应用充分说明了电场诱导的侧带和贴头的连贯性以及BLOCH状态散射之间的相互作用。准颗粒带的处理方式完全笼统地处理,允许任意形式的内在旋转轨道耦合(SOC),并可以扩展到外部SOC。根据先前的结果,在存在疾病潜力的情况下,除了整个费米海引起的固有贡献外,带有带中的带间响应,除其他效果外,浆果曲率对波动行动动力学的贡献还包括散射引起的异常贡献,这对Fermi表面的存在敏感。为了证明我们的理论捕获的丰富物理学,考虑了不同强度顺序的放松时间矩阵,同时我们明确求解了简单无序的Rashba模型的某些电场响应属性,这些响应属性由频带间相干性贡献主导。我们提出的表达式适合数值计算,我们通过对带间贡献的完整带结构计算(即使在金属中)进行完整的带结构计算来证明这一点。

We present a general formalism for investigating the second-order optical response of solids to an electric field in weakly disordered crystals with arbitrarily complicated band structures based on density-matrix equations of motion, on a Born approximation treatment of disorder, and on an expansion in scattering rate to leading non-trivial order. One of the principal aims of our work is to enable extensive transport theory applications that accounts fully for the interplay between electric-field-induced interband and intraband coherence, and Bloch-state scattering. The quasiparticle bands are treated in a completely general manner that allows for arbitrary forms of the intrinsic spin-orbit coupling (SOC) and could be extended to the extrinsic SOC. According to the previous results, in the presence of the disorder potential, the interband response in conductors in addition to an intrinsic contribution due to the entire Fermi sea that captures, among other effects, the Berry curvature contribution to wave-packet dynamics includes an anomalous contribution caused by scattering that is sensitive to the presence of the Fermi surface. To demonstrate the rich physics captured by our theory, the relaxation time matrix for different strength order is considered and at the same time we explicitly solve for some electric-field response properties of simple disordered Rashba model that are known to be dominated by interband coherence contributions. The expressions we present are amenable for numerical calculations, and we demonstrate this by performing a full band-structure calculation of the interband contribution, even in metals.

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