论文标题

探测温度诱导的单个铁电域壁的相变

Probing temperature-induced phase transitions at individual ferroelectric domain walls

论文作者

Kelley, Kyle P., Kalinin, Sergei V., Eliseev, Eugene, Raghuraman, Shivaranjan, Jesse, Stephen, Maksymovych, Peter, Morozovska, Anna N.

论文摘要

由于它们表现出的功能行为的广泛差异,铁电域壁已成为凝结物理学中最迷人的物体中最迷人的物体之一。但是,绝大多数域壁研究都集中在偏见引起的动态和运输行为上。在这里,我们介绍了基于压电响应力显微镜(PFM)的扫描探针显微镜方法,并与动态加热探针结合了局部加热和材料的局部偏见。这种方法用于探索软SN2P2S6铁电的热极化动力学,并允许探索各个域壁上的相变。引入了热PFM的强和弱调制状态。讨论了加热探针方法在功能性SPM测量中的未来潜在应用,包括压电,弹性,微波和运输测量。

Ferroelectric domain walls have emerged as one of the most fascinating objects in condensed matter physics due to the broad variability of functional behaviors they exhibit. However, the vast majority of domain walls studies have been focused on bias-induced dynamics and transport behaviors. Here, we introduce the scanning probe microscopy approach based on piezoresponse force microscopy (PFM) with a dynamically heated probe, combining local heating and local biasing of the material. This approach is used to explore the thermal polarization dynamics in soft Sn2P2S6 ferroelectrics, and allows for the exploration of phase transitions at individual domain walls. The strong and weak modulation regimes for the thermal PFM are introduced. The future potential applications of heated probe approach for functional SPM measurements including piezoelectric, elastic, microwave, and transport measurements are discussed.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源