论文标题

量子在有限温度下机械驱动的结构旋转玻璃

Quantum mechanically driven structural-spin glass in two dimensions at finite temperature

论文作者

Hotta, Chisa, Ueda, Kazumasa, Imada, Masatoshi

论文摘要

在磁性材料中,旋转有时会冻结成空间无序的玻璃状态。在三个维度上经常发现形成液体或结构玻璃的玻璃。但是,在两个维度(2D)中,据信,自旋玻璃和结构玻璃在有限温度下永远不可能存在,因为它们被热波动破坏。使用大规模的量子蒙特卡洛模拟,我们在有限温度下发现了量子力学驱动的2D玻璃相。我们的平台是一个iSing自旋模型,在沮丧的三角形晶格上具有量子横向场。以下三个步骤可以理解当前玻璃相的形成。首先,通过几何挫败感和量子波动的相互作用,旋转的一部分自发地形成了抗磁性蜂窝状自旋 - 旋转体系结构。然后,键相互作用中的小随机性是对该上层建筑的相关扰动,并将其分解为{\ it域},使其成为结构性玻璃。上层建筑的玻璃又产生了作用在剩余的波动旋转上并冻结的新出现的随机磁场。因此形成的域的形状取决于淬灭过程,这是玻璃的特征之一,源自多谷利自由能景观。当前的系统仅由{\ ut}单一的自由度组成,自然而然地,它不是单独成为结构性玻璃,也不是单独的旋转玻璃。然而,具有两种类型性质的玻璃以共存的两个组成玻璃,代数结构玻璃和远距离有序的旋转玻璃的形式出现。这种新的玻璃形成机制概念即使在低维系统中也可以实现功能性眼镜。

In magnetic materials, spins sometimes freeze into spatially disordered glassy states. Glass forming liquids or structural glasses are found very often in three dimensions. However, in two dimensions(2D) it is believed that both spin glass and structural glass can never exist at a finite temperature because they are destroyed by thermal fluctuations. Using a large-scale quantum Monte Carlo simulation, we discover a quantum-mechanically driven 2D glass phase at finite temperatures. Our platform is an Ising spin model with a quantum transverse field on a frustrated triangular lattice. How the present glass phase is formed is understood by the following three steps. First, by the interplay of geometrical frustration and quantum fluctuation, part of the spins spontaneously form an antiferromagnetic honeycomb spin-superstructure. Then, small randomness in the bond interaction works as a relevant perturbation to this superstructure and breaks it up into {\it domains}, making it a structural glass. The glassiness of the superstructure, in turn, generates an emergent random magnetic field acting on the remaining fluctuating spins and freezes them. The shape of domains thus formed depends sensitively on the quenching process, which is one of the characteristic features of glass, originating from a multi-valley free-energy landscape. The present system consists only of {\it a single} bistable Ising degree of freedom, which naturally does not become a structural glass alone nor a spin glass alone. Nevertheless, a glass having both types of nature emerges in the form of coexisting two-component glasses, algebraic structural-glass and long-range ordered spin-glass. This new concept of glass-forming mechanism opens a way to realize functional glasses even in low dimensional systems.

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