论文标题

时间逆转对称性破坏电荷密度的CSV $ _3 $ SB $ _5 $由Polar Kerr效应检测到

Time-reversal symmetry breaking in charge density wave of CsV$_3$Sb$_5$ detected by polar Kerr effect

论文作者

Hu, Yajian, Yamane, Soichiro, Mattoni, Giordano, Yada, Kanae, Obata, Keito, Li, Yongkai, Yao, Yugui, Wang, Zhiwei, Wang, Jingyuan, Farhang, Camron, Xia, Jing, Maeno, Yoshiteru, Yonezawa, Shingo

论文摘要

由于其独特的几何特性,Kagome晶格表现出丰富的量子现象。有吸引力的实现是Kagome金属AV $ _3 $ SB $ _5 $(A = K,RB,CS),在该k,rb,cs)中,非常规的电荷密度波(CDW)与超导性和非平凡的乐队拓扑交织在一起。几个实验表明,这种CDW是罕见的手性CDW,其特征是轨道环电流。但是,环电流,自发的时间反转对称性(TRSB)以及其阶参数与磁场的耦合仍然难以捉摸。在这里,我们通过磁光极性Kerr效应和亚微分辨率研究了CSV3SB5中的CDW。在磁场下,我们观察到CDW过渡时Kerr角的跳跃。这种跳跃是磁场可切换的,并用场缩放,表明与非平凡带拓扑相关的磁性耦合。在零场,我们发现CDW过渡温度以下的非零和磁场可训练的KERR角,信号自发TRSB。我们的结果为揭示相关的kagome材料中的量子现象提供了至关重要的步骤。

The Kagome lattice exhibits rich quantum phenomena owing to its unique geometric properties. Appealing realizations are the Kagome metals AV$_3$Sb$_5$ (A = K, Rb, Cs), where unconventional charge density wave (CDW) is intertwined with superconductivity and non-trivial band topology. Several experiments suggest that this CDW is a rare occurrence of chiral CDW characterized by orbital loop current. However, key evidences of loop current, spontaneous time-reversal symmetry-breaking (TRSB) and the coupling of its order parameter with the magnetic field remain elusive. Here, we investigate the CDW in CsV3Sb5 by magneto-optic polar Kerr effect with sub-microradian resolution. Under magnetic field, we observed a jump of the Kerr angle at the CDW transition. This jump is magnetic-field switchable and scales with field, indicating magneto--chirality coupling related to non-trivial band topology. At zero field, we found non-zero and field-trainable Kerr angle below CDW transition temperature, signaling spontaneous TRSB. Our results provide a crucial step to unveil quantum phenomena in correlated Kagome materials.

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