论文标题

Kagome Metal(CS,RB)v $ _3 $ SB $ _5 $中的订单disorder peierls不稳定

Order-disorder Peierls instability in the kagome metal (Cs,Rb)V$_3$Sb$_5$

论文作者

Subires, D., Korshunov, A., Said, A. H., Sánchez, L., Ortiz, Brenden R., Wilson, Stephen D., Bosak, A., Blanco-Canosa, S.

论文摘要

kagome金属化合物AV $ _3 $ SB $ _5 $中电荷密度波阶段的性质提出了许多问题,其起源仍在争论中。在这里,我们结合了散射散射(DS)和非弹性X射线散射(IXS),以识别电荷阶的3维(3D)前体与传播载体(0.5 0 0.5),通过一阶相变凝结成3D-CDW。准弹性临界散射表明对扩散前体的主要贡献是弹性中心峰,而没有声子软化。然而,非弹性光谱显示在接近相变时,爱因斯坦型声子模式的宽扩大很小。我们的结果指出了\ textIt {l}点的费米表面不稳定性的情况是订单disorder类型,具有准静态域的临界增长。结果超出了经典的弱耦合PEIERLS过渡动力学,并在包括强电子耦合和非绝热性在内的模型中进行了讨论。

The nature of the charge density wave phases in the kagome metal compound AV$_3$Sb$_5$ has raised many questions and their origin is still under debate. Here, we combine diffuse scattering (DS) and inelastic x-ray scattering (IXS) to identify a 3-dimensional (3D) precursor of the charge order with propagation vector (0.5 0 0.5), which condenses into a 3D-CDW through a first order phase transition. The quasi-elastic critical scattering indicates that the dominant contribution to the diffuse precursor is the elastic central peak without phonon softening. However, the inelastic spectra show a small broadening of the Einstein-type phonon mode on approaching the phase transition. Our results point to the situation where the Fermi surface instability at the \textit{L} point is of order-disorder type with a critical growth of quasi-static domains. The results go beyond the classical weak-coupling Peierls transition dynamics and are discussed within models including strong-electron phonon coupling and non-adiabaticity.

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