论文标题
致密乳液中分形景观动力学的实验观察
Experimental observations of fractal landscape dynamics in a dense emulsion
论文作者
论文摘要
许多柔软的生物材料都表现出所谓的“软玻璃”动力学;他们的成分会发生异常的随机运动和复杂的合作重排。一种最近对一种软玻璃材料的模拟模型,一种粗化的泡沫,表明其气泡的随机运动是由于系统构型在高维空间中的分形能量景观上移动。在这里,我们表明,可以使用来自许多自由度的经验轨迹数据,以无模型的方式探索和可靠地探索此类高维分形景观的显着几何特征。对于类似蛋黄酱的密度乳液,对所观察到的油滴轨迹的分析可定量再现构型路径的高维分形几何形状及其使用计算模型产生的相关能量最小值。这种几何形状又驱动了在真实空间中观察到的液滴的复杂随机运动。我们的结果表明,实验研究可以阐明不同软和生物材料中类似的动力学是否也可能是由于分形景观动力学引起的。
Many soft and biological materials display so-called 'soft glassy' dynamics; their constituents undergo anomalous random motions and complex cooperative rearrangements. A recent simulation model of one soft glassy material, a coarsening foam, suggested that the random motions of its bubbles are due to the system configuration moving over a fractal energy landscape in high-dimensional space. Here we show that the salient geometrical features of such high-dimensional fractal landscapes can be explored and reliably quantified, using empirical trajectory data from many degrees of freedom, in a model-free manner. For a mayonnaise-like dense emulsion, analysis of the observed trajectories of oil droplets quantitatively reproduces the high-dimensional fractal geometry of the configuration path and its associated energy minima generated using a computational model. That geometry in turn drives the droplets' complex random motion observed in real space. Our results indicate that experimental studies can elucidate whether the similar dynamics in different soft and biological materials may also be due to fractal landscape dynamics.