论文标题

基于多物理模拟和数据驱动的替代模型,优化SOEC的同质性和效率

Optimizing the Homogeneity and Efficiency of an SOEC Based on Multiphysics Simulation and Data-driven Surrogate Model

论文作者

Chi, Yingtian, Yokoo, Kentaro, Nakajima, Hironori, Ito, Kohei, Lin, Jin, Song, Yonghua

论文摘要

不均匀的电流和温度分布对固体氧化物电解电池(SOEC)的耐用性有害。分段的SOEC实验表明,有利于系统效率的高蒸汽利用可导致局部蒸汽饥饿并增强不均匀性。在优化研究中,有必要考虑共同考虑不均匀性和效率。通过实验验证的三维(3D)多物理模型可以以可靠的方式模拟不均匀性,但由于高计算成本,它们不适合优化。这项研究提出了一种结合分段的SOEC实验,多物理模拟和人工智能的方法,以优化共同的SOEC的不均匀性和效率。首先通过分段的SOEC实验构建和验证3D细胞模型。然后,快速神经网络替代模型是根据仿真数据构建的,并集成到多目标优化问题中。它的解决方案形成了帕累托阵线,反映了不同目标之间的冲突关系。发现当蒸汽利用率为0.7时,下游电流为上流电流的60%-65%。为了将蒸汽利用率提高到0.8,下游电流将进一步下降到上流电流的50%-60%。帕累托前线使系统操作员能够在效率和不均匀性之间达到平衡。

Inhomogeneous current and temperature distributions are harmful to the durability of the solid oxide electrolysis cell (SOEC). Segmented SOEC experiments reveal that a high steam utilization, which is favorable for system efficiency, leads to local steam starvation and enhanced the inhomogeneity. It is necessary to consider inhomogeneity and efficiency jointly in optimization studies. Three-dimensional (3D) multiphysics models validated with experiments can simulate the inhomogeneity in a reliable manner, but they are unsuitable for optimization due to the high computational cost. This study proposes a method that combines segmented SOEC experiments, multiphysics simulation, and artificial intelligence to optimize the inhomogeneity and efficiency of SOEC jointly. A 3D cell model is first built and verified by segmented SOEC experiments. Then, fast neural network surrogate models are built from the simulation data and integrated into a multi-objective optimization problem. Its solutions form a Pareto front reflecting the conflicting relationships among different objectives. It is found that the down-stream current is 60%-65% of the up-stream current when the steam utilization is 0.7. To increase the steam utilization to 0.8, the down-stream current will further drop to 50%-60% of the up-stream current. The Pareto fronts enable system operators to achieve a balance between efficiency and inhomogeneity.

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