论文标题

水稳定的MOF和疏水封装的MOF,可从环境空气和湿烟气中捕获二氧化碳

Water-stable MOFs and Hydrophobically Encapsulated MOFs for CO2 Capture from Ambient Air and Wet Flue Gas

论文作者

Shi, Xiaoyang, Lee, Gahyun Annie, Liu, Shuohan, Kim, Dongjae, Alahmed, Ammar, Jamal, Aqil, Wang, Lei, Park, Ah-Hyung Alissa

论文摘要

已经释放到大气中的额外二氧化碳必须被去除,以创造一个碳中性的世界。已经创建了从湿烟气或直接从环境空气中去除二氧化碳的技术,但是这些技术尚未被广泛部署。由于最近改善了材料组装和表面化学的改善,因此已经产生了新一代的创意二氧化碳捕获吸附剂。我们总结了在广泛的环境和操作条件下捕获二氧化碳框架(MOF)的最新进展。特别是,讨论了新发达的水稳定的MOF和疏水涂料技术,并深入了解其材料发现以及这些混合吸附系统的不同组件之间的协同作用。还给出了从湿烟气中直接捕获二氧化碳和二氧化碳捕获的水稳定和封装的MOF的未来观点和方向。

The extra CO2 that has already been released into the atmosphere has to be removed in order to create a world that is carbon neutral. Technologies have been created to remove carbon dioxide from wet flue gas or even directly from ambient air, however these technologies are not widely deployed yet. New generations of creative CO2 capture sorbents have been produced as a consequence of recent improvements in material assembly and surface chemistry. We summarize recent progress on water-stable and encapsulated metal-organic frameworks (MOFs) for CO2 capture under a wide range of environmental and operating conditions. In particular, newly developed water-stable MOFs and hydrophobic coating technologies are discussed with insights into their materials discovery and the synergistic effects between different components of these hybrid sorbent systems. The future perspectives and directions of water-stable and encapsulated MOFs are also given for Direct Air Capture of CO2 and CO2 capture from wet flue gas.

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