论文标题

电荷密度波的结构la $ _ {1.875} $ ba $ _ {0.125} $ cuo $ _4 $

Structure of Charge Density Waves in La$_{1.875}$Ba$_{0.125}$CuO$_4$

论文作者

Sears, J., Shen, Y., Krogstad, M. J., Miao, H., Bozin, E. S., Robinson, I. K., Gu, G. D., Osborn, R., Rosenkranz, S., Tranquada, J. M., Dean, M. P. M.

论文摘要

尽管在几个库酸酯超级传播家族中存在电荷密度波(CDW)相关性,但它们在CDW波形和相关长度方面表现出很大的变化,表明CDW晶格相互作用的关键作用。我们在LA $ _ {1.875} $ ba $ _ {0.125} $ cuo $ _4 $的情况下调查了这种交互,使用单晶X射线衍射来收集大量CDW峰强度,并确定了Cu和La/ba the-la/ba原子扭曲。在CUO $ _2 $飞机中,扭曲涉及沿订购波矢量方向的Cu-Cu间距的定期调制。铜氧层内的电荷顺序诱导周围灯笼层的平面外呼吸调节,这会导致相邻的铜氧层的相关变形。我们的结果暗示,与CDW相关的结构扭曲不局限于单层,而是通过晶体传播明显的距离。这导致了重叠的结构调制,其中CuO $ _2 $飞机表现出由相邻层的正交CDW以及层本身内CDW的变形引起的畸变。我们将这种引人注目的效果归因于铜层中的弱C轴电荷筛选,并表明这种效果可以帮助将CDW与晶体中相邻平面之间的CDW相结合。

Although charge-density wave (CDW) correlations exist in several families of cuprate supercon-ductors, they exhibit substantial variation in CDW wavevector and correlation length, indicating a key role for CDW-lattice interactions. We investigated this interaction in La$_{1.875}$Ba$_{0.125}$CuO$_4$ using single crystal x-ray diffraction to collect a large number of CDW peak intensities, and determined the Cu and La/Ba atomic distortions induced by the formation of CDW order. Within the CuO$_2$ planes, the distortions involve a periodic modulation of the Cu-Cu spacing along the direction of the ordering wave vector. The charge ordering within the copper-oxygen layer induces an out-of-plane breathing modulation of the surrounding lanthanum layers, which leads to a related distortion on the adjacent copper-oxygen layer. Our result implies that the CDW-related structural distortions do not remain confined to a single layer but rather propagate an appreciable distance through the crystal. This leads to overlapping structural modulations, in which CuO$_2$ planes exhibit distortions arising from the orthogonal CDWs in adjacent layers as well as distortions from the CDW within the layer itself. We attribute this striking effect to the weak c-axis charge screening in cuprates and suggest this effect could help couple the CDW between adjacent planes in the crystal.

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