论文标题
电荷密度波的结构la $ _ {1.875} $ ba $ _ {0.125} $ cuo $ _4 $
Structure of Charge Density Waves in La$_{1.875}$Ba$_{0.125}$CuO$_4$
论文作者
论文摘要
尽管在几个库酸酯超级传播家族中存在电荷密度波(CDW)相关性,但它们在CDW波形和相关长度方面表现出很大的变化,表明CDW晶格相互作用的关键作用。我们在LA $ _ {1.875} $ ba $ _ {0.125} $ cuo $ _4 $的情况下调查了这种交互,使用单晶X射线衍射来收集大量CDW峰强度,并确定了Cu和La/ba the-la/ba原子扭曲。在CUO $ _2 $飞机中,扭曲涉及沿订购波矢量方向的Cu-Cu间距的定期调制。铜氧层内的电荷顺序诱导周围灯笼层的平面外呼吸调节,这会导致相邻的铜氧层的相关变形。我们的结果暗示,与CDW相关的结构扭曲不局限于单层,而是通过晶体传播明显的距离。这导致了重叠的结构调制,其中CuO $ _2 $飞机表现出由相邻层的正交CDW以及层本身内CDW的变形引起的畸变。我们将这种引人注目的效果归因于铜层中的弱C轴电荷筛选,并表明这种效果可以帮助将CDW与晶体中相邻平面之间的CDW相结合。
Although charge-density wave (CDW) correlations exist in several families of cuprate supercon-ductors, they exhibit substantial variation in CDW wavevector and correlation length, indicating a key role for CDW-lattice interactions. We investigated this interaction in La$_{1.875}$Ba$_{0.125}$CuO$_4$ using single crystal x-ray diffraction to collect a large number of CDW peak intensities, and determined the Cu and La/Ba atomic distortions induced by the formation of CDW order. Within the CuO$_2$ planes, the distortions involve a periodic modulation of the Cu-Cu spacing along the direction of the ordering wave vector. The charge ordering within the copper-oxygen layer induces an out-of-plane breathing modulation of the surrounding lanthanum layers, which leads to a related distortion on the adjacent copper-oxygen layer. Our result implies that the CDW-related structural distortions do not remain confined to a single layer but rather propagate an appreciable distance through the crystal. This leads to overlapping structural modulations, in which CuO$_2$ planes exhibit distortions arising from the orthogonal CDWs in adjacent layers as well as distortions from the CDW within the layer itself. We attribute this striking effect to the weak c-axis charge screening in cuprates and suggest this effect could help couple the CDW between adjacent planes in the crystal.